Recent Progress on Graphene-Based Flexible All-Solid-State Supercapacitors

doi:10.11944/j.issn.1000-0518.2018.03.170381

Chinese Journal of Applied Chemistry ›› 2018, Vol. 35 ›› Issue (3): 259-271.DOI: 10.11944/j.issn.1000-0518.2018.03.170381

• Review • Previous Articles Next Articles

Recent Progress on Graphene-Based Flexible All-Solid-State Supercapacitors

LI Ning,CHEN Tao()

Institute of Advanced Study,School of Chemical Science and Engineering,Tongji University,Shanghai 200092,China

Received:2017-10-26 Accepted:2017-12-13 Published:2018-03-05 Online:2018-02-12
Contact: CHEN Tao
Supported by:
Supported by the National Natural Science Foundation of China(No.51503152, No.51702237), the Shanghai Rising-Star Program(No.17QA1404300), the Program for Professor of Special Appointment(Eastern Scholar) at Shanghai Institutions of Higher Learning, and the Youth Talent Support Program at Shanghai

Abstract

Abstract:

With the development of electronics towards intelligence, portability and miniaturization, it is necessary to develop high-performance flexible energy storage devices. Due to their high power density, long cycling life, excellent safety, environmentally-friend, and easy realization of flexibility, supercapacitors have attracted increasing attention recently. Graphene-based materials, exhibiting large specific surface area, excellent electrochemical performance and superior mechanical stability, have been widely investigated as electrode materials in flexible all-solid-state supercapacitors. In this review, we introduce the fabrications of graphene-based electrodes, and summarize recent progress on flexible all-solid-state supercapacitors followed by discussing perspective and current challenges of this hot field.

Key words: graphene, flexibility, all-solid-state, supercapacitor

LI Ning, CHEN Tao. Recent Progress on Graphene-Based Flexible All-Solid-State Supercapacitors[J]. Chinese Journal of Applied Chemistry, 2018, 35(3): 259-271.

References

[1]	Rogers J A,Someya T,Huang Y G.Materials and Mechanics for Stretchable Electronics[J]. Science,2010,327(5973):1603-1607.
[2]	Ramuz M,Tee B C K,Tok J B H,et al. Transparent, Optical, Pressure-sensitive Artificial Skin for Large-area Stretchable Electronics[J]. Adv Mater,2012,24(24):3223-3227.
[3]	Majumder S,Mondal T,Deen M J.Wearable Sensors for Remote Health Monitoring[J]. Sensors,2017,17(1):130.
[4]	Larson C,Peele B,Li S,et al.Highly Stretchable Electroluminescent Skin for Optical Signaling and Tactile Sensing[J]. Science,2016,351(6277):1071-1074.
[5]	Weng W,Chen P N,He S S,et al.Smart Electronic Textiles[J]. Angew Chem Int Ed,2016,55(21):6140-6169.
[6]	Gao Y,Ota H,Schaler E W,et al.Wearable Microfluidic Diaphragm Pressure Sensor for Health and Tactile Touch Monitoring[J]. Adv Mater,2017,29(39):1701985.
[7]	Xie K Y,Wei B Q.Materials and Structures for Stretchable Energy Storage and Conversion Devices[J]. Adv Mater,2014,26(22):3592-3617.
[8]	Hu Y H,Sun X L.Flexible Rechargeable Lithium Ion Batteries:Advances and Challenges in Materials and Process Technologies[J]. J Mater Chem A,2014,2(28):10712-10738.
[9]	Chen T,Peng H S,Durstock M,et al.High-performance Transparent and Stretchable All-solid Supercapacitors Based on Highly Aligned Carbon Nanotube Sheets[J]. Sci Rep,2014,4:3612.
[10]	Lv T,Yao Y,Li N,et al.Wearable Fiber-shaped Energy Conversion and Storage Devices Based on Aligned Carbon Nanotubes[J]. Nano Today,2016,11(5):644-660.
[11]	Chen T,Dai L M.Flexible Supercapacitors Based on Carbon Nanomaterials[J]. J Mater Chem A,2014,2(28):10756-10775.
[12]	Lv T,Yao Y,Li N,et al.Highly Stretchable Supercapacitors Based on Aligned Carbon Nanotube/Molybdenum Disulfide Composites[J]. Angew Chem Int Ed,2016,55(32):9191-9195.
[13]	Chen T,Hao R,Peng H S,et al.High-Performance, Stretchable, Wire-shaped Supercapacitors[J]. Angew Chem Int Ed,2015,54(2):618-622.
[14]	Wen L,Li F,Cheng H M.Carbon Nanotubes and Graphene for Flexible Electrochemical Energy Storage: From Materials to Devices[J]. Adv Mater,2016,28(22):4306-4337.
[15]	Ren W C,Cheng H M.The Global Growth of Graphene[J]. Nat Nanotechnol,2014,9(10):726-730.
[16]	Bonaccorso F,Colombo L,Yu G H,et al.Graphene, Related Two-dimensional Crystals, and Hybrid Systems for Energy Conversion and Storage[J]. Science,2015,347(6217):1246501.
[17]	Li N,Lv T,Yao Y,et al.Compact Graphene/MoS2 Composite Films for Highly Flexible and Stretchable All-solid-state Supercapacitors[J]. J Mater Chem A,2017,5(7):3267-3273.
[18]	Xiao F,Yang S X,Zhang Z Y,et al.Scalable Synthesis of Freestanding Sandwich-structured Graphene/Polyaniline/Graphene Nanocomposite Paper for Flexible All-solid-state Supercapacitor[J]. Sci Rep,2015,5:9359.
[19]	Dong Y F,Wu Z S,Ren W C,et al.Graphene:A Promising 2D Material for Electrochemical Energy Storage[J]. Sci Bull,2017,62(10):724-740.
[20]	Novoselov K S,Fal'ko V I,Colombo L,et al. A Roadmap for Graphene[J]. Nature,2012,490(7419):192-200.
[21]	Xu Z,Peng L,Liu Y J,et al.Experimental Guidance to Graphene Macroscopic Wet-spun Fibers, Continuous Papers, and Ultralightweight Aerogels[J]. Chem Mater,2017,29(1):319-330.
[22]	Xu Z,Gao C.Graphene Fiber:A New Trend in Carbon Fibers[J]. Mater Today,2015,18(9):480-492.
[23]	Yang Z B,Sun H,Chen T,et al.Photovoltaic Wire Derived from a Graphene Composite Fiber Achieving an 8.45% Energy Conversion Efficiency[J]. Angew Chem Int Ed,2013,52(29):7545-7548.
[24]	Meng F C,Lu W B,Li Q W,et al.Graphene-based Fibers:A Review[J]. Adv Mater,2015,27(35):5113-5131.
[25]	Xu Z,Liu Y J,Zhao X L,et al.Ultrastiff and Strong Graphene Fibers via Full-scale Synergetic Defect Engineering[J]. Adv Mater,2016,28(30):6449-6456.
[26]	Xu Z,Gao C.Graphene Chiral Liquid Crystals and Macroscopic Assembled Fibres[J]. Nat Commun,2011,2:571.
[27]	Liu Y J,Xu Z,Zhan J M,et al.Superb Electrically Conductive Graphene Fibers via Doping Strategy[J]. Adv Mater,2016,28(36):7941-7947.
[28]	Xin G Q,Yao T K,Sun H T,et al.Highly Thermally Conductive and Mechanically Strong Graphene Fibers[J]. Science,2015,349(6252):1083-1087.
[29]	Li X M,Zhao T S,Wang K L,et al.Directly Drawing Self-assembled, Porous, and Monolithic Graphene Fiber from Chemical Vapor Deposition Grown Graphene Film and Its Electrochemical Properties[J]. Langmuir,2011,27(19):12164-12171.
[30]	Chen T,Dai L M.Macroscopic Graphene Fibers Directly Assembled from CVD-grown Fiber-shaped Hollow Graphene Tubes[J]. Angew Chem Int Ed,2015,54(49):14947-14950.
[31]	Eda G,Fanchini G,Chhowalla M.Large-area Ultrathin Films of Reduced Graphene Oxide as a Transparent and Flexible Electronic Material[J]. Nat Nanotechnol,2008,3(5):270-274.
[32]	Eigler S,Enzelberger-Heim M,Grimm S,et al.Wet Chemical Synthesis of Graphene[J]. Adv Mater,2013,25(26):3583-3587.
[33]	Liu L H,Lyu J,Zhao T K,et al.Large Area Preparation of Multilayered Graphene Films by Chemical Vapour Deposition with High Electrocatalytic Activity Toward Hydrogen Peroxide[J]. Mater Technol,2015,30(A3):A121-A126.
[34]	Kumar P,Shahzad F,Yu S,et al.Large-area Reduced Graphene Oxide Thin Film with Excellent Thermal Conductivity and Electromagnetic Interference Shielding Effectiveness[J]. Carbon,2015,94:494-500.
[35]	Xiong Z Y,Liao C L,Han W H,et al.Mechanically Tough Large-area Hierarchical Porous Graphene Films for High-performance Flexible Supercapacitor Applications[J]. Adv Mater,2015,27(30):4469-4475.
[36]	Zhang M,Huang L,Chen J,et al.Ultratough, Ultrastrong, and Highly Conductive Graphene Films with Arbitrary Sizes[J]. Adv Mater,2014,26(45):7588-7592.
[37]	Peng L,Xu Z,Liu Z,et al.Ultrahigh Thermal Conductive yet Superflexible Graphene Films[J]. Adv Mater,2017,29(27):1700589.
[38]	Kim K S,Zhao Y,Jang H,et al.Large-scale Pattern Growth of Graphene Films for Stretchable Transparent Electrodes[J]. Nature,2009,457(7230):706-710.
[39]	Li X S,Cai W W,An J H,et al.Large-area Synthesis of High-quality and Uniform Graphene Films on Copper Foils[J]. Science,2009,324(5932):1312-1314.
[40]	Wang M,Jang S K,Jang W J,et al.A Platform for Large-scale Graphene Electronics-CVD Growth of Single-layer Graphene on CVD-grown Hexagonal Boron Nitride[J]. Adv Mater,2013,25(19):2746-2752.
[41]	Tan R K L,Reeves S P,Hashemi N,et al. Graphene as a Flexible Electrode:Review of Fabrication Approaches[J]. J Mater Chem A,2017,5(34):17777-17803.
[42]	Jiang W,Xin H,Li W.Microcellular 3D Graphene Foam via Chemical Vapor Deposition of Electroless Plated Nickel Foam Templates[J]. Mater Lett,2016,162:105-109.
[43]	Deng W,Fang Q L,Zhou X F,et al.Hydrothermal Self-assembly of Graphene Foams with Controllable Pore Size[J]. RSC Adv,2016,6(25):20843-20849.
[44]	Liu T,Huang M L,Li X F,et al.Highly Compressible Anisotropic Graphene Aerogels Fabricated by Directional Freezing for Efficient Absorption of Organic Liquids[J]. Carbon,2016,100:456-464.
[45]	Zhang Q Q,Zhang F,Medarametla S P,et al.3D Printing of Graphene Aerogels[J]. Small,2016,12(13):1702-1708.
[46]	Lv J L,Meng Y,Suzuki K,et al.Fabrication of 3D Graphene Foam for a Highly Conducting Electrode[J]. Mater Lett,2017,196:369-372.
[47]	Chen Z P,Ren W C,Gao L B,et al.Three-dimensional Flexible and Conductive Interconnected Graphene Networks Grown by Chemical Vapour Deposition[J]. Nat Mater,2011,10(6):424-428.
[48]	Du X S,Liu H Y,Mai Y W.Ultrafast Synthesis of Multifunctional N-Doped Graphene Foam in an Ethanol Flame[J]. ACS Nano,2016,10(1):453-462.
[49]	Lv L X,Zhang P P,Cheng H H,et al.Solution-processed Ultraelastic and Strong Air-bubbled Graphene Foams[J]. Small,2016,12(24):3229-3234.
[50]	Zhu Y W,Murali S,Stoller M D,et al.Carbon-based Supercapacitors Produced by Activation of Graphene[J]. Science,2011,332(6037):1537-1541.
[51]	Zhu J Y,Childress A S,Karakaya M,et al.Defect-engineered Graphene for High-energy- and High-power-density Supercapacitor Devices[J]. Adv Mater,2016,28(33):7185-7192.
[52]	Wu Z S,Winter A,Chen L,et al.Three-dimensional Nitrogen and Boron Co-doped Graphene for High-performance All-solid-state Supercapacitors[J]. Adv Mater,2012,24(37):5130-5135.
[53]	Choi B G,Chang S J,Kang H W,et al.High Performance of a Solid-state Flexible Asymmetric Supercapacitor Based on Graphene Films[J]. Nanoscale,2012,4(16):4983-4988.
[54]	El-Kady M F,Strong V,Dubin S,et al. Laser Scribing of High-performance and Flexible Graphene-based Electrochemical Capacitors[J]. Science,2012,335(6074):1326-1330.
[55]	Chen X L,Lin H J,Deng J,et al.Electrochromic Fiber-shaped Supercapacitors[J]. Adv Mater,2014,26(48):8126-8132.
[56]	Yang Z B,Deng J,Chen X L,et al.A Highly Stretchable, Fiber-shaped Supercapacitor[J]. Angew Chem Int Ed,2013,52(50):13453-13457.
[57]	Hu Y,Cheng H H,Zhao F,et al.All-in-One Graphene Fiber Supercapacitor[J]. Nanoscale,2014,6(12):6448-6451.
[58]	Yu D S,Goh K,Wang H,et al.Scalable Synthesis of Hierarchically Structured Carbon Nanotube-graphene Fibres for Capacitive Energy Storage[J]. Nat Nanotechnol,2014,9(7):555-562.
[59]	Zhao X L,Zheng B N,Huang T Q,et al.Graphene-based Single Fiber Supercapacitor with a Coaxial Structure[J]. Nanoscale,2015,7(21):9399-9404.
[60]	Luo Y F,Zhang Y,Zhao Y,et al.Aligned Carbon Nanotube/Molybdenum Disulfide Hybrids for Effective Fibrous Supercapacitors and Lithium Ion Batteries[J]. J Mater Chem A,2015,3(34):17553-17557.
[61]	Sheng L Z,Wei T,Liang Y,et al.Vertically Oriented Graphene Nanoribbon Fibers for High-volumetric Energy Density All-solid-state Asymmetric Supercapacitors[J]. Small,2017,13(22):1700371.
[62]	Meng Y N,Zhao Y,Hu C G,et al.All-graphene Core-sheath Microfibers for All-solid-state, Stretchable Fibriform Supercapacitors and Wearable Electronic Textiles[J]. Adv Mater,2013,25(16):2326-2331.
[63]	Kou L,Huang T Q,Zheng B N,et al.Coaxial Wet-spun Yarn Supercapacitors for High-energy Density and Safe Wearable Electronics[J]. Nat Commun,2014,5:3754.
[64]	Chen S B,Wang L,Huang M M,et al.Reduced Graphene Oxide/Mn3O4 Nanocrystals Hybrid Fiber for Flexible All-solid-state Supercapacitor with Excellent Volumetric Energy Density[J]. Electrochim Acta,2017,242:10-18.
[65]	Ding X T,Zhao Y,Hu C G,et al.Spinning Fabrication of Graphene/Polypyrrole Composite Fibers for All-solid-state, Flexible Fibriform Supercapacitors[J]. J Mater Chem A,2014,2(31):12355-12360.
[66]	Qu G X,Cheng J L,Li X D,et al.A Fiber Supercapacitor with High Energy Density Based on Hollow Graphene/Conducting Polymer Fiber Electrode[J]. Adv Mater,2016,28(19):3646-3652.
[67]	Sun G Z,Zhang X,Lin R Z,et al.Hybrid Fibers Made of Molybdenum Disulfide, Reduced Graphene Oxide, and Multi-walled Carbon Nanotubes for Solid-State, Flexible, Asymmetric Supercapacitors[J]. Angew Chem Int Ed,2015,54(15):4651-4656.
[68]	Zhang D,Miao M,Niu H,et al.Core-Spun Carbon Nanotube Yarn Supercapacitors for Wearable Electronic Textiles[J]. ACS Nano,2014,8(5):4571-4579.
[69]	Yao B,Zhang J,Kou T Y,et al.Paper-based Electrodes for Flexible Energy Storage Devices[J]. Adv Sci,2017,4(7):1700107.
[70]	Mosa I M,Pattammattel A,Kadimisetty K,et al.Ultrathin Graphene-protein Supercapacitors for Miniaturized Bioelectronics[J]. Adv Energy Mater,2017,7(17):1700358.
[71]	Peng L L,Peng X,Liu B R,et al.Ultrathin Two-dimensional MnO2/Graphene Hybrid Nanostructures for High-performance, Flexible Planar Supercapacitors[J]. Nano Lett,2013,13(5):2151-2157.
[72]	Chen T,Dai L M.Carbon Nanomaterials for High-performance Supercapacitors[J]. Mater Today,2013,16(7/8):272-280.
[73]	Bettini L G,Galluzzi M,Podesta A,et al.Planar Thin Film Supercapacitor Based on Cluster-assembled Nanostructured Carbon and Ionic Liquid Electrolyte[J]. Carbon,2013,59:212-220.
[74]	Yoo J J,Balakrishnan K,Huang J S,et al.Ultrathin Planar Graphene Supercapacitors[J]. Nano Lett,2011,11(4):1423-1427.
[75]	Li M,Tang Z,Leng M,et al.Flexible Solid-state Supercapacitor Based on Graphene-based Hybrid Films[J]. Adv Funct Mater,2014,24(47):7495-7502.
[76]	Li F W,Chen J T,Wang X S,et al.Stretchable Supercapacitor with Adjustable Volumetric Capacitance Based on 3D Interdigital Electrodes[J]. Adv Funct Mater,2015,25(29):4601-4606.
[77]	Jo K,Lee S,Kim S M,et al.Stacked Bilayer Graphene and Redox-active Interlayer for Transparent and Flexible High-performance Supercapacitors[J]. Chem Mater,2015,27(10):3621-3627.
[78]	Wu Z S,Zheng Y J,Zheng S H,et al.Stacked-layer Heterostructure Films of 2D Thiophene Nanosheets and Graphene for High-rate All-solid-state Pseudocapacitors with Enhanced Volumetric Capacitance[J]. Adv Mater,2017,29(3):1602960.
[79]	Chen T,Xue Y H,Roy A K,et al.Transparent and Stretchable High-performance Supercapacitors Based on Wrinkled Graphene Electrodes[J]. ACS Nano,2014,8(1):1039-1046.
[80]	Hong J Y,Kim W,Cho D,et al.Omnidirectionally Stretchable and Transparent Graphene Electrodes[J]. ACS Nano,2016,10(10):9446-9455.
[81]	Xu Y,Lin Z,Huang X,et al.Flexible Solid-State Supercapacitors Based on Three-Dimensional Grahene Hydrogel Films[J]. ACS Nano,2013,7(5):4042-4049.
[82]	Yuan K,Guo-Wang P,Hu T,et al.Nanofibrous and Graphene-templated Conjugated Microporous Polymer Materials for Flexible Chemosensors and Supercapacitors[J]. Chem Mater,2015,27(21):7403-7411.
[83]	Yuan K,Hu T,Xu Y,et al.Engineering the Morphology of Carbon Materials:2D Porous Carbon Nanosheets for High-performance Supercapacitors[J]. ChemElectroChem,2016,3(5):822-828.
[84]	Yuan K,Xu Y,Uihlein J,et al.Straightforward Generation of Pillared, Microporous Graphene Frameworks for Use in Supercapacitors[J]. Adv Mater,2015,27(42):6714-6721.
[85]	Qi D,Liu Y,Liu Z,et al.Design of Architectures and Materials in In-plane Micro-supercapacitors:Current Status and Future Challenges[J]. Adv Mater,2017,29(5):1602802.
[86]	Kyeremateng N A,Brousse T,Pech D.Microsupercapacitors as Miniaturized Energy-storage Components for On-chip Electronics[J]. Nat Nanotechnol,2017,12(1):7-15.
[87]	Liu L L,Niu Z Q,Chen J.Design and Integration of Flexible Planar Micro-supercapacitors[J]. Nano Res,2017,10(5):1524-1544.
[88]	Huang P,Lethien C,Pinaud S,et al.On-chip and Freestanding Elastic Carbon Films for Micro-supercapacitors[J]. Science,2016,351(6274):691-695.
[89]	Yun J,Kim D,Lee G,et al.All-solid-state Flexible Micro-supercapacitor Arrays with Patterned Graphene/MWNT Electrodes[J]. Carbon,2014,79:156-164.
[90]	Yu W,Zhou H,Li B Q,et al.3D Printing of Carbon Nanotubes-based Microsupercapacitors[J]. ACS Appl Mater Interfaces,2017,9(5):4597-4604.
[91]	Li J T,Delekta S S,Zhang P P,et al.Scalable Fabrication and Integration of Graphene Microsupercapacitors Through Full Inkjet Printing[J]. ACS Nano,2017,11(8):8249-8256.
[92]	Liu Z Y,Wu Z S,Yang S,et al.Ultraflexible In-plane Micro-supercapacitors by Direct Printing of Solution-processable Electrochemically Exfoliated Graphene[J]. Adv Mater,2016,28(11):2217-2222.
[93]	El-Kady M F,Kaner R B. Scalable Fabrication of High-power Graphene Micro-supercapacitors for Flexible and On-chip Energy Storage[J]. Nat Commun,2013,4:1475.
[94]	Zhang L,DeArmond D,Alvarez N T,et al. Flexible Micro-supercapacitor Based on Graphene with 3D Structure[J]. Small,2017,13(10):1603114.
[95]	Wu Z S,Parvez K,Feng X L,et al.Graphene-based In-plane Micro-supercapacitors with High Power and Energy Densities[J]. Nat Commun,2013,4:2487.
[96]	Liu Z Y,Liu S H,Dong R H,et al.High Power In-plane Micro-supercapacitors Based on Mesoporous Polyaniline Patterned Graphene[J]. Small,2017,13(14):1603388.
[97]	Zhang P P,Zhu F,Wang F X,et al.Stimulus-responsive Micro-supercapacitors with Ultrahigh Energy Density and Reversible Electrochromic Window[J]. Adv Mater,2017,29(7):1604491.
[98]	Qi D P,Liu Z Y,Liu Y,et al.Suspended Wavy Graphene Microribbons for Highly Stretchable Microsupercapacitors[J]. Adv Mater,2015,27(37):5559-5566.

Recent Progress on Graphene-Based Flexible All-Solid-State Supercapacitors

RichHTML

PDF

Knowledge

Cited

Abstract

Cite this article

share this article

References

Related Articles 15

Recommended Articles

Metrics

Comments

[1]	Yue-Hua ZHAO, Da-Peng WANG. Coadsorption Kinetics of Amino‑Functionalized Graphene Oxide and Fatty Acids at the Water/Oil Interface [J]. Chinese Journal of Applied Chemistry, 2022, 39(8): 1274-1284.
[2]	Wen-Dong WANG, Zai-Jun LI. Synthesis of Ruthenium‑Graphene Quantum Dots Artificial Oxidase and Its Application in Colorimetric Detection of Phoxim in Carrots [J]. Chinese Journal of Applied Chemistry, 2022, 39(8): 1285-1293.
[3]	Shan SHAO, Jian ZHANG, Kai-Qiang DENG, Jie YANG, Shao-Ming YANG. Detection of Dopamine by Enzyme‑Free Sensor Constructed by Nickel‑Cobalt Bimetallic‑porphyrin Organic Framework Composites [J]. Chinese Journal of Applied Chemistry, 2022, 39(7): 1098-1107.
[4]	Qing-Fang NIU, Xin AI, Yi-Xuan WANG, Fang-Jiu HE, Bi LUO, Wen-Ting LIANG, Chuan DONG. Synthesis of Three‑Dimensional Reduced Graphene Oxide/β‑Cyclodextrin Complex and Its Electrochemical Detection of Levofloxacin in Water [J]. Chinese Journal of Applied Chemistry, 2022, 39(7): 1129-1137.
[5]	Qiao-Zhi GUO, Zhen-Hua YANG, Yue-Xia ZHANG, Ya-Ting MENG, Yu-Juan CAO, Xuan-Sen SUN, Qi-Qi ZHANG, Shao-Min SHUANG, Chuan DONG. Synthesis and Applications of Graphene Quantum Dots Derived from Citric Acid [J]. Chinese Journal of Applied Chemistry, 2022, 39(6): 888-899.
[6]	Yi-Xin XU, Shuang WANG, Jing QUAN, Wan-Ting GAO, Tian-Qun SONG, Mei YANG. Preparation of Molybdenum Disulfide Quantum Dots/Reduced Graphene Oxide Composites and Their Photocatalytic Degradation of Organic Dyes， Tetracyclines and Cr（VI） [J]. Chinese Journal of Applied Chemistry, 2022, 39(5): 769-778.
[7]	LIU Wen-Bin, YANG Sha-Sha, HUANG Guo-Lin, FAN Li-Jiao, XIE Yu-Ming. Synthesis of Phosphorylated Xanthan Gum/Graphene Oxide and Its Selective Adsorption of Uranium [J]. Chinese Journal of Applied Chemistry, 2021, 38(6): 658-667.
[8]	ZHANG Ya-Jing, WANG Xiao-Hui, XU Ya-Juan, LIU Wen-Shu, ZHAO Li-Hui. Preparation of Graphene Nano-Drug Carrier System and Its Killing Effect on Tumor Cells [J]. Chinese Journal of Applied Chemistry, 2021, 38(6): 693-703.
[9]	GAO Feng, XU Zi-Di, GUAN Chun-Qian, WANG Yan, ZANG Yun-Hao, QU Jiang-Ying. Green Controllable Synthesis of Sulfur/Graphene Aerogel and Performance of Lithium Sulfur Battery [J]. Chinese Journal of Applied Chemistry, 2021, 38(4): 439-446.
[10]	XIAO Haimei, CAI Lei, ZHANG Zhaohui, CHEN Shan, ZHOU Shu, FU Jinli. Preparation of Ion-Imprinted Polymers Based on Magnetic Graphene Oxide/MIL-101 (Cr) and Selective Adsorption of Cu(Ⅱ) and Pb(Ⅱ) [J]. Chinese Journal of Applied Chemistry, 2020, 37(9): 1076-1086.
[11]	GAO Siheng, YANG Yu, WU Jinling, QIN Lixia, KANG Shizhao, LI Xiangqing. Preparation and Photoelectric Performance of Graphene Oxide/Ultrafine Silver Composite [J]. Chinese Journal of Applied Chemistry, 2020, 37(8): 923-929.
[12]	SI Xiaojing, ZHU Wenjing, LI Xiang, LI Li, CHEN Zichao, DING Yaping. Determination of Ofloxacin in Medicine via Poly(p-aminobenzene sulfonic acid)/Graphene Electrochemical Modified Electrode [J]. Chinese Journal of Applied Chemistry, 2020, 37(6): 726-732.
[13]	FAN Zhe,ZHANG Shengsheng,TANG Jiahao,FAN Ping. Structure, Preparation and Application of Graded Nanomaterials [J]. Chinese Journal of Applied Chemistry, 2020, 37(5): 489-501.
[14]	ZHANG Xiaobo, XIN Haiying, XU Shuang, ZHANG Xinghai, WANG Liqiu. Cellulose Gel Polymer Electrolytes and Its Application in Supercapacitors [J]. Chinese Journal of Applied Chemistry, 2020, 37(5): 547-554.
[15]	LIU Xue, MA Hua, XU Heng, JI Haicong, WANG Dong. Lithium Storage Properties of Non-woven Fabric Based Polypyrrole Flexible Electrodes [J]. Chinese Journal of Applied Chemistry, 2020, 37(5): 555-561.