Fabrication of Succinic Acid Anhydride Grafted Cellulose Nanofiber Membrane and Its Adsorption of Heavy Metal Ions

doi:10.11944/j.issn.1000-0518.2017.08.160299

Chinese Journal of Applied Chemistry ›› 2017, Vol. 34 ›› Issue (8): 891-898.DOI: 10.11944/j.issn.1000-0518.2017.08.160299

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Fabrication of Succinic Acid Anhydride Grafted Cellulose Nanofiber Membrane and Its Adsorption of Heavy Metal Ions

CHEN Peizhen^a^*(),LIU Ruilai^a^b,ZHAO Jinyun^a,RAO Ruiye^a

^a Fujian Provincial Key laboratory of Eco-Industrial Green Technology,College of Ecological and Resources Engineering,Wuyi University,Wuyishan,Fujian 354300,China
^b Fujian Provincial Key Laboratory of Polymer Materials,College of Material Science and Engineering,Fujian Normal University,Fuzhou 350007,China

Received:2016-07-22 Accepted:2016-10-14 Published:2017-07-25 Online:2017-07-26
Contact: CHEN Peizhen
Supported by:
Supported by the National Natural Science Foundation of China(No.51406141), JK Project of Fujian Educational Bureau(No 2014052, No.2012055), Natural Science Foundation of Nanping Science and Technology Bureau(No.2011DJ10)

Abstract

Abstract:

Triacetate cellulose(TCA) porous nanofiber membranes(Cell) with diameter of (110±28) nm were successfully prepared by thermally induced phase separation. Succinic acid anhydride grafted cellulose(Cell-g-SAA) nanofiber membranes were obtained through hydrolyzation and grafting of TCA nanofibers. The Cell and Cell-g-SAA membranes were used for the adsorption of Cu²⁺ and Pb²⁺. The adsorption kinetics and thermodynamics were studied and found to fit pseudo-second-order and Langmuir model. Compared with cellulose membranes, the max adsorption capacity of Cell-g-SAA membranes for Cu²⁺ and Pb²⁺ increases from 51.73 and 34.29 mg/g to 116.41 and 51.73 mg/g, respectively. The adsorptions of Cu²⁺ and Pb²⁺ on the Cell and Cell-g-SAA membranes are more agreeable with monolayer adsorption mode via mainly chemical interactions.

Key words: succinic acid anhydride, grafting, nanofibers, heavy metal, adsorption

CHEN Peizhen, LIU Ruilai, ZHAO Jinyun, RAO Ruiye. Fabrication of Succinic Acid Anhydride Grafted Cellulose Nanofiber Membrane and Its Adsorption of Heavy Metal Ions[J]. Chinese Journal of Applied Chemistry, 2017, 34(8): 891-898.

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Fabrication of Succinic Acid Anhydride Grafted Cellulose Nanofiber Membrane and Its Adsorption of Heavy Metal Ions

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