Chinese Journal of Applied Chemistry ›› 2024, Vol. 41 ›› Issue (3): 391-404.DOI: 10.19894/j.issn.1000-0518.230278
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Yuan-Jie LI1, Bing-Bing FAN1, Jun-Li ZHANG2(), Yan-Mei ZHOU1()
Received:
2023-09-13
Accepted:
2024-01-25
Published:
2024-03-01
Online:
2024-04-09
Contact:
Jun-Li ZHANG,Yan-Mei ZHOU
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CLC Number:
Yuan-Jie LI, Bing-Bing FAN, Jun-Li ZHANG, Yan-Mei ZHOU. Research Progress in the Application of Amino Acid Ionic Liquids to Energy Storage and Biomass Resource Utilization[J]. Chinese Journal of Applied Chemistry, 2024, 41(3): 391-404.
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Group | Cations of AA-PILs |
---|---|
Aromatic amino acids | |
Hetetocuclic amino acid | |
Aliphatic amino acid |
Table 1 Cations and anions ([HSO4]-) of 21 AA-PILs.
Group | Cations of AA-PILs |
---|---|
Aromatic amino acids | |
Hetetocuclic amino acid | |
Aliphatic amino acid |
Fig.3 (a) SEM of [Lys][HSO4]2 precursor carbon material; (b, c) SEM of Lys-K2CO3 ([Lys][HSO4]2 carbon material activated by K2CO3; (d-f) N, O and S heteroatom distributions of Lys-K2CO3[44]; (g) SEM of [HSO4] precursor carbon material; (h, i)SEM of Asn-5-NaHCO3 (Asn carbon material modulated with NaHCO3 by the addition of sodium dodecyl sulfate at a mass traction of 5%); (j-l) N, O and S heteroatom distribution of Asn-5-NaHCO3[50]
Fig.4 (a) Schematic of the synthesis of L-lysine-assisted cubic nitrogen-doped ordered mesoporous carbon material (ArRF-700); (b, c) SEM images of ArRF-700 at different magnifications[41]; (d, e) HR-SEM electron microscopy images of CIL(Tyr)-C; (f) HR-TEM electron microscopy images of CIL(Tyr)-C[63]
Entry | Catalyst | Substrate | Reaction dosage | Product | Yield | ||
---|---|---|---|---|---|---|---|
Solvent | Temperature/℃ | Time | |||||
1 | [Cho][Pro][ | glucose | H2O | 80 | 30 min | Fructose | 37.6% |
2 | [Lys][HSO4]2[ | glucose | [Bmim][Cl] | 130 | 1.5 h | Total reducing sugars | 67.1% |
3 | TyrPTA-Ag[ | cellulose | H2O | 140 | 1.5 h | Total reducing sugars | 71.3% |
4 | Tyrosine oxalate[ | wheat straw | H2O | 90 | 3 h | Total reducing sugars | 86.3% |
5 | [TBA][Arg][ | sunflower oil | Methanol n(methanol)∶n(oil)=9∶1 | 90 | 15 min | Biodiesel | 98.8% |
6 | [N2222][Arg][ | soybean oil | Methanol n(methanol)∶n(oil)=10∶1 | 100 | 60 min | Biodiesel | 98.4% |
7 | [Cly][Cl][ | rice straw | H2O | 37 | 40 d | CH4 | 115.56 mg/g |
Table 2 Application of AA-ILs in catalytic conversion of biomass
Entry | Catalyst | Substrate | Reaction dosage | Product | Yield | ||
---|---|---|---|---|---|---|---|
Solvent | Temperature/℃ | Time | |||||
1 | [Cho][Pro][ | glucose | H2O | 80 | 30 min | Fructose | 37.6% |
2 | [Lys][HSO4]2[ | glucose | [Bmim][Cl] | 130 | 1.5 h | Total reducing sugars | 67.1% |
3 | TyrPTA-Ag[ | cellulose | H2O | 140 | 1.5 h | Total reducing sugars | 71.3% |
4 | Tyrosine oxalate[ | wheat straw | H2O | 90 | 3 h | Total reducing sugars | 86.3% |
5 | [TBA][Arg][ | sunflower oil | Methanol n(methanol)∶n(oil)=9∶1 | 90 | 15 min | Biodiesel | 98.8% |
6 | [N2222][Arg][ | soybean oil | Methanol n(methanol)∶n(oil)=10∶1 | 100 | 60 min | Biodiesel | 98.4% |
7 | [Cly][Cl][ | rice straw | H2O | 37 | 40 d | CH4 | 115.56 mg/g |
Fig.5 (a) AA-PILs catalyzes hydrolysis of cellulose to produce total reducing sugar[75]; (b) TyrPTA-Ag catalyzes hydrolysis of cellulose to produce total reducing sugar[76]
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