Preparation and Characterization of ZnMgAl Hydrotalcite Supported BiOI

doi:10.11944/j.issn.1000-0518.2019.01.180059

Chinese Journal of Applied Chemistry ›› 2019, Vol. 36 ›› Issue (1): 83-90.DOI: 10.11944/j.issn.1000-0518.2019.01.180059

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Preparation and Characterization of ZnMgAl Hydrotalcite Supported BiOI

LI Jiaqi^a,FU Dayou^a^*(),YUAN Dong^b,XU Jing^b

^aCollege of Chemical Engineering
^bCollege of Chemistry and Environmental Engineering,Sichuan University of Science and Engineering,Zigong,Sichuan 643000,China

Received:2018-03-06 Accepted:2018-06-26 Published:2019-01-01 Online:2019-01-04
Contact: FU Dayou
Supported by:
Supported by the Science & Technology Department of Sichuan Province(No.2013JY0081), the Innovation Fund of Postgraduate, Sichuan University of Science and Engineering(No.y2018057), the Green Catalysis Key Laboratory Open Fund Project of Universities in Sichuan Province(No.LYJ1405)

Abstract

Abstract:

The ZnMgAl hydrotalcite-like compounds(HTLCs) supported bismuth oxyiodide(BiOI)(BiOI/ZnMgAl-HTLCs) visible light photocatalyst was prepared by hydrothermal method. The effects of BiOI loading mass fraction, reaction temperature, reaction time, and addition sequence on the structure and morphology of the BiOI/ZnMgAl-HTLCs photocatalyst were investigated by X-ray diffraction(XRD), scanning electron microscopy(SEM) and Fourier transform infrared spectroscopy(FTIR). The results show that BiOI/ZnMgAl-HTLCs with high crystallinity and good morphology can be obtained by firstly adding BiOI in 40% mass fraction to ZnMgAl-HTLCs at 140 ℃, and keeping reaction for 24 h.

Key words: ZnMgAl hydrotalcite-like compounds, bismuth oxyiodide, photocatalyst

LI Jiaqi, FU Dayou, YUAN Dong, XU Jing. Preparation and Characterization of ZnMgAl Hydrotalcite Supported BiOI[J]. Chinese Journal of Applied Chemistry, 2019, 36(1): 83-90.

References

[1]	Wang L J,Wang L R,Feng Y J,et al. Highly Efficient and Selective Infrared Absorption Material Based on Layered Double Hydroxides for Use in Agricultural Plastic Film[J]. Appl Clay Sci,2011,53(4):592-597.
[2]	Wang L J,Xu X Y,Evans D G,et al. Synthesis and Selective IR Absorption Properties of Iminodiacetic-Acid Intercalated MgAl-layered Double Hydroxide[J]. J Solid State Chem,2010,183(5):1114-1119.
[3]	Evants D G,Rct S.Structure Aspects of Layered Double Hydroxide[J]. Struct Bond,2006,119:1-87.
[4]	Zhu H F,Tang P G,Feng Y J,et al. Intercalation of IR Absorber into Layered Double Hydroxides:Preparation, Thermal Stability and Selective IR Absorption[J]. Mater Res Bull,2012,47(3):532-536.
[5]	Li L D,Yu J J,Hao Z P,et al. Novel Ru-Mg-Al-O Catalyst Derived from Hydrotalcite-Like Compound for NO Storage/Decomposition/Reduction[J]. J Phys Chem C,2007,111(28):10552-10559.
[6]	Obalová L,Jirátová K,Kovanda F,et al. Catalytic Decomposition of Nitrous Oxide over Catalysts Prepared from Co/Mg-Mn/Al Hydrotalcite-like Compounds[J]. Appl Catal B-Environ,2005,60:289-297.
[7]	Shao M,Ning F,Zhao J,et al. Preparation of Fe3O4/SiO2/Layered Double Hydroxide Coreshell Microspheres for Magnetic Separation of Proteins[J]. J Am Chem Soc,2012,134:1071-1077.
[8]	Lu X,Wang G,Zhai T,et al. Hydrogenated TiO2 Nanotube Arrays for Supercapacitors[J]. Nano Lett,2012,12:1690-1696.
[9]	Yuan D,Zhou L,Fu D Y,et al. Adsorption of Methyl Orange from Aqueous Solutions by Calcined ZnMgAl Hydrotalcite[J]. Appl Phys A-Mater,2017,123:146-153.
[10]	Xu J Y,Liu J,Li K D,et al. Novel PEPA-Functionalized Graphene Oxide for Fire Safety Enhancement of Polypropylene[J]. Sci Technol Adv Mater,2015,(16):1-11.
[11]	Song Y,Wang J,Li Z,et al. Self-assembled Hierarchical Porous Layered Double Hydroxides by Solvothermal Method and Their Application for Capacitors[J]. Micropor Mesopor Mater,2012,148(1):159-165.
[12]	Zhang L,Zhang X,Shen L,et al. Enhanced High-Current Capacitive Behavior of Graphene/CoAl-layered Double Hydroxide Composites as Electrode Material for Supercapacitors[J]. J Power Sources,2012,199:395-401.
[13]	Hou W G,Jin Z L.Synthesis and Characterization of Naproxen Intercalated Zn-Al Layered Double Hydroxides[J]. Colloid Polym Sci,2007,285(13):1449-1454.
[14]	XUE Yuanming,FAN Lihui,LIU Dongbin,et al. Photocatalytic Degradation of Methyl Orange on ZnCr Layered Double Hydroxides[J]. J Shenyang Univ Chem Tech,2015,29(3):233-237(in Chinese). 薛源明,樊丽辉,刘东斌,等. 锌铬水滑石可见光降解甲基橙的性能研究[J]. 沈阳化工大学学报,2015,29(3):233-237.
[15]	WANG Lina.Prepapation and Properties of Go/BiOI Composite Visible-Light Photocatalytic Materials[D]. Harbin:Harbin Normal University,2013(in Chinese). 王丽娜. GO/BiOI复合可见光催化材料的制备及性能研究[D]. 哈尔滨:哈尔滨师范大学,2013.
[16]	Chen L,Huang R,Xiong M,et al. Room-Temperature Synthesis of Flower-Like BiOX(X=Cl,Br,I) Hierarchical Structures and Their Visible-Light Photocatalytic Activity[J]. Inorg Chem,2013,52(19):11118-11125.
[17]	Liu Q C,Ma D K,Hu Y Y,et al. Various Bismuth Oxyiodide Hierarchical Architectures:Alcohothermal-Controlled Synthesis, Photocatalytic Activities, and Adsorption Capabilities for Phosphate in Water[J]. ACS Appl Mater Interfaces,2013,5(22):11927-11934.
[18]	WANG Na,ZHONG Jianchu,WANG Hongzhi,et al. Preparation, Characterization and Application of Calcium and Aluminum Layered Double Hydroxides Intercalated by Boric Acid Radical[J]. Inorg Chem Ind,2016,48(1):25-27(in Chinese). 王娜,仲剑初,王洪志. 硼酸根插层的Ca-Al-LDHs的制备、表征和应用[J]. 无机盐工业,2016,48(1):25-27.
[19]	WANG Ruirui.Studies on Synthesis and Properties of Layered Double Hydroxides Intercalated with Drugs[D]. Harbin:Harbin Engineering University,2012(in Chinese). 王瑞瑞. 药物插层水滑石复合材料的制备与性能研究[D]. 哈尔滨:哈尔滨工程大学,2012.
[20]	Wang J T,Xu F.Preparation of EDTA Pillared MgZnAl LDHs and Its Adsorption of Pb(Ⅱ)[J]. Chem Res Appl,2014,26(4):581-585.
[21]	Han X G,He H Z,Kuang Q,et al. Controlling Morphologies and Tuning the Related Properties of Nano/Microstructured ZnO Crystallites[J]. J Phys Chem C,2009,113(2):584-589.

Preparation and Characterization of ZnMgAl Hydrotalcite Supported BiOI

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